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ElectrolysisHigh temperatureIndustrial scaleCO₂-emitting

Hall-Héroult process

Electrolysis at 950-980 °C of alumina dissolved in molten cryolite (Na₃AlF₆) to produce aluminium metal. Universal since 1886 — it alone consumes ~3 % of world electricity.

Decomposition driven by electric current

Key reaction

2 Al₂O₃ + 3 C → 4 Al + 3 CO₂ (anode consommable, ~13 kWh/kg)

Operating conditions

Temperature
950-980°C
Pressure
1bar
Catalyst
Cryolithe Na₃AlF₆ fondue + AlF₃ + CaF₂
Phase
liquid

How it works

Schema coming soon

How it works

Aluminium metal cannot be produced by conventional carbothermic reduction: its oxide Al₂O₃ is too stable (ΔG_f = −1582 kJ/mol). The solution, found simultaneously by Charles Hall (USA) and Paul Héroult (France) in 1886, is electrolysis in a molten cryolite bath. A modern Hall-Héroult cell is ~10 × 4 m, holds ~25 cm of liquid bath at 950-980 °C, and runs at 4-4.5 V for currents of 200,000 to 600,000 A (recent AP60-type plants exceed 600 kA). The cathode is a carbon lining at the cell bottom; anodes are carbon blocks (~1.5 × 0.7 × 0.5 m) suspended in the bath and gradually lowered as they're consumed. Alumina, fed to the bath by automatic injection, dissolves as oxofluoroaluminates (AlOF₂⁻, Al₂OF₆²⁻). At the cathode, liquid aluminium deposits (density 2.3 > bath at 2.1 — Al accumulates at the bottom and is siphoned every 24 h). At the anode, the oxygen released immediately attacks the carbon: that's why anodes are consumable and the process emits CO₂. The overall balance is: 2 Al₂O₃ + 3 C → 4 Al + 3 CO₂. Theoretical electrical consumption is 5.99 kWh/kg Al; best modern plants run at 12.5-13 kWh/kg Al, an energy efficiency of ~46 %. World production is ~70 Mt/year (2023), dominated by China (~60 %) — where electricity is largely coal-fired, making Chinese aluminium particularly carbon-intensive (~16 t CO₂/t Al vs ~4 t CO₂/t Al for Icelandic or Quebec hydroelectric aluminium).

Key components

The role of each main part, and the elements / compounds it involves.

  • Reduction cell (pot)

    Electrolysis reactor — holds the molten cryolite bath and the liquid aluminium produced.

    Rectangular cell ~10 × 4 × 1.2 m, steel shell internally lined with carbon blocks (cathode) then an insulating frozen-alumina crust. The cell tilts slightly and a siphon draws off the molten Al collected at the bottom. A modern plant lines up 200-300 cells in series, forming a 'potline' fed by a single giant rectifier.

    10 × 4 × 1,2 m · 200-600 kA · 4-4,5 V · 200-300 cuves en série

  • Carbon anodes

    Supply electrons and are consumed by reaction with the released oxygen.

    Pre-baked carbon blocks (Söderberg technology nearly extinct) made from calcined petroleum coke + coal-tar pitch, baked at 1200 °C. ~1.5 × 0.7 × 0.5 m, ~1 t each. A cell holds 20-30 anodes, replaced every 25-30 days. Consumption: ~400 kg carbon per tonne Al — this is what makes the process an irreducible CO₂ emitter (at least ~1.5 t CO₂/t Al just from the anodes).

    Coke Pb + brai · cuit 1200 °C · ~400 kg C/t Al · changement /25-30 j

  • Electrolytic bath (cryolite + AlF₃)

    Molten ionic solvent that dissolves alumina and carries current between anode and cathode.

    Na₃AlF₆ (cryolite) + AlF₃ (8-12 % excess) + CaF₂ (~5 %) + 2-4 % dissolved Al₂O₃. This composition lowers the melting point of Al₂O₃ from 2050 °C to ~960 °C — the central trick of the process. Natural cryolite (Greenland) being exhausted, it's synthesized from fluorspar + hydrofluoric acid. Fluoride losses: 15-25 kg F/t Al — partially captured by the off-gas treatment system.

    Na₃AlF₆ + 8-12 % AlF₃ + 5 % CaF₂ · Tf ~960 °C · 2-4 % Al₂O₃

    See also :al2o3
  • Alumina feeders

    Automatically deliver alumina to the bath to maintain 2-4 % dissolution.

    Pneumatic dosers injecting 1-2 kg of Al₂O₃ every 1-3 minutes per cell, controlled by bath resistance (which rises as alumina depletes). Below 1 %, the 'anode effect' kicks in: high voltage, formation of PFCs (CF₄, C₂F₆) — greenhouse gases 6,500-9,200× more potent than CO₂. Fine control is therefore climate-critical.

    1-2 kg/min · contrôle par résistance · seuil 1 % critique (PFC)

    See also :al2o3
  • Tapping siphon

    Withdraws the molten aluminium pooled at the cell bottom without stopping electrolysis.

    Refractory steel tube lowered into the cell from the top, set under suction by a vacuum bell. Tapping of 1-2 t Al at 950 °C in 5-15 min, ~24 times/day. Tapped Al still contains 0.1-0.3 % impurities (Fe, Si) and is then refined in a holding furnace before casting into ingots, billets or plates.

    1-2 t/cuve/coulée · ~24×/jour · 0,1-0,3 % impuretés résiduelles

Physical and chemical principles

The fundamental laws that make this process possible — and the constraints they impose.

  • Electrochemical decomposition

    Theoretical decomposition potential of Al₂O₃ is 1.18 V at 977 °C. Real voltage (4-4.5 V) includes anode and cathode overpotentials, ohmic drop in the bath, and connection resistance. The gap is where energy inefficiency sits — hence the constant effort on geometry and bath quality.

    E°(977 °C) = 1,18 V ; U_industrielle = 4-4,5 V
  • Thermal stability of the bath

    Joule heating (R·I²) of the current in the bath produces the heat that keeps it molten. The cell runs at a precarious thermal equilibrium: too hot, the carbon lining erodes; too cold, alumina stops dissolving and the anode effect kicks in. A frozen-alumina 'crust' on the walls acts as a buffering thermal insulator.

    Applies to components :cuve-electrolysebain-cryolithe

Compounds involved

World production

70 Mt/yr
2023

Main applications

  • Transportation (automotive, aerospace, rail)28 %
  • Construction (frames, façades)25 %
  • Packaging (cans, foils)17 %
  • Electrical (overhead lines, conductors)12 %
  • Machinery, durables, miscellaneous18 %

Decarbonizing aluminium

Primary aluminium emits ~13-16 t CO₂/t Al (global average mix), i.e. 2 % of global industrial emissions. Three major levers are being pursued: (1) inert anodes made of ceramic oxide or refractory metal that don't burn off and release O₂ instead of CO₂ — Elysis demonstrators (Rio Tinto/Alcoa) being scaled up, (2) low-carbon electricity (hydro, nuclear, renewables) which can cut the footprint by 4×, (3) recycling: remelting aluminium uses only 5 % of the energy of primary production.
  • Anodes inertes (Elysis, RUSAL) — démonstrateurs 450 kA
  • Hall-Héroult bas-carbone (Islande, Norvège, Québec)
  • Cellules de très grande taille (600+ kA, AP60)
  • Boucle de recyclage post-consumer (97 % de récupération sur les canettes)

Similar or competing processes

Related industrial processes — alternative chemistry, alternative technology.

  • bayer

    Upstream process — supplies the pure alumina that Hall-Héroult electrolyses.

History and discovery

Discovery year1886
First industrial deployment1888
Charles Martin Hall · Paul Héroult· États-Unis / France
Sources
  • Grjotheim, K. — Aluminium Electrolysis: Fundamentals of the Hall-Héroult Process
  • International Aluminium Institute — Statistical Reports
  • USGS Mineral Commodity Summaries — Aluminum
  • IEA — Aluminium Tracking Report
Processes